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Optoplasmonic materials that contain both metallic (plasmonic) and dielectric building blocks can sustain synergistic
electromagnetic interactions between photonic and plasmonic resonances and, thus, pave the way to overcoming the
limitations of the respective building blocks. A significant challenge in realizing the full potential of these unique
electromagnetic materials is the integration of building blocks with different chemical compositions and sizes into
defined morphologies. We demonstrate in this paper that template guided self-assembly strategies show great promise in
realizing intricate discrete and extended optoplasmonic materials. Selected examples of optoplasmonic materials and the
underlying fabrication methods are discussed. The first example combines dielectric microspheres as whispering gallery
mode resonators with plasmonic antennas. The latter are located at defined locations in close vicinity of (but not attached
to) the dielectric microsphere. The interactions of WGMs with plasmonic resonators located in their evanescent field are
analyzed. The second example describes two-dimensional interdigitated arrays of 250 nm diameter TiO2 NPs and
clusters of electromagnetically strongly coupled 60 nm gold nanoparticles. It is demonstrated that delocalized photonic–
plasmonic modes in the arrays achieve a cascaded E-field enhancement in the gap junctions of the gold NP clusters.
Yan Hong,Wonmi Ahn,Xin Zhao, andBjörn M. Reinhard
"Template-guided self-assembly strategies for discrete and extended optoplasmonic materials", Proc. SPIE 9374, Advanced Fabrication Technologies for Micro/Nano Optics and Photonics VIII, 93740Q (13 March 2015); https://doi.org/10.1117/12.2076065
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Yan Hong, Wonmi Ahn, Xin Zhao, Björn M. Reinhard, "Template-guided self-assembly strategies for discrete and extended optoplasmonic materials," Proc. SPIE 9374, Advanced Fabrication Technologies for Micro/Nano Optics and Photonics VIII, 93740Q (13 March 2015); https://doi.org/10.1117/12.2076065