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22 August 2020 Oligonucleotide guided plasmonic nanocavity for quasi-deterministic quantum strong coupling
Shiuan-Yeh Chen, Jyun-Hong Chen, Hao-Yu Liu, Wei-Lun Chou, Wen-Yuan Chen, Wan-Pin Chan
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Proceedings Volume 11462, Plasmonics: Design, Materials, Fabrication, Characterization, and Applications XVIII; 114620J (2020) https://doi.org/10.1117/12.2567854
Event: SPIE Nanoscience + Engineering, 2020, Online Only
Abstract
Quantum strong coupling between emitters and cavities generates hybrid modes which provide a platform for quantum devices. The atom based systems require precise control over the position of atoms within the cavity and are difficult to be integrated on a chip. The quantum dots-photonic crystal system is limited to the cryogenic temperature. On the contrary, the molecule-plasmonic cavity is a good candidate for chip scale, room temperature operating strong coupling units due to the extremely small mode volume of plasmonic nanocavities. However, to precisely position a single or a few molecules into a plasmonic nanocavity is challenging. In this work, a few molecules are integrated into the nanocavity through oligonucleotides. The clear Rabi splitting is observed and the anti-crossing curve shows a clear verification of coupling. The number of fluorophore integrated into the nanocavity is estimated to be one. The deterministic strong coupling may be realized based on this configuration.
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Shiuan-Yeh Chen, Jyun-Hong Chen, Hao-Yu Liu, Wei-Lun Chou, Wen-Yuan Chen, and Wan-Pin Chan "Oligonucleotide guided plasmonic nanocavity for quasi-deterministic quantum strong coupling", Proc. SPIE 11462, Plasmonics: Design, Materials, Fabrication, Characterization, and Applications XVIII, 114620J (22 August 2020); https://doi.org/10.1117/12.2567854
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KEYWORDS
Plasmonics
Molecules
Chemical species
Control systems
Crystals
Cryogenics
Estimation theory
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