15 January 1990 Optical Third Harmonic Measurements Of Macrocyclic Conjugated Chains
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Abstract
The third order optical susceptibilities X(3)1111(-3ω;ω,ω,ω) for the macrocyclic conjugated structural class of annulenes with an 18-28 membered ring size were determined systematically by optical third harmonic generation measurements of molecularly doped polymer films at a wavelength of 1.907 μm. The X(3)1111/N values are found to possess a power law dependence with increased size of the annulenes.
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T. Wada, T. Wada, J. Ojima, J. Ojima, A. Yamada, A. Yamada, A. F. Garito, A. F. Garito, H. Sasabe, H. Sasabe, } "Optical Third Harmonic Measurements Of Macrocyclic Conjugated Chains", Proc. SPIE 1147, Nonlinear Optical Properties of Organic Materials II, (15 January 1990); doi: 10.1117/12.962133; https://doi.org/10.1117/12.962133
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