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Using ultrafast double-pulse spectroscopy, our experiment showcases coherent control over the 2.39 THz optical phonon mode within bulk WTe2. Through precise manipulation of the delay between successive pump pulses, we successfully achieve modulation of the phonon amplitude at room temperature by a factor of two. This breakthrough showcases the potential for all-optical control and modulation of the unique properties in WTe2 that are directly bound to its structural degrees of freedom.
Conference Presentation
(2023) Published by SPIE. Downloading of the abstract is permitted for personal use only.
Sergio I. Rey P.,Martin J. Cross,Malte L. Welsch,Tobias O. Buchmann,Binbin Zhou,Peter U. Jepsen, andEdmund J. R. Kelleher
"All-optical control of coherent phonons in the candidate type-II Weyl semimetal WTe2", Proc. SPIE 12681, Ultrafast Nonlinear Imaging and Spectroscopy XI, 126810A (5 October 2023); https://doi.org/10.1117/12.2690825
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Sergio I. Rey P., Martin J. Cross, Malte L. Welsch, Tobias O. Buchmann, Binbin Zhou, Peter U. Jepsen, Edmund J. R. Kelleher, "All-optical control of coherent phonons in the candidate type-II Weyl semimetal WTe2," Proc. SPIE 12681, Ultrafast Nonlinear Imaging and Spectroscopy XI, 126810A (5 October 2023); https://doi.org/10.1117/12.2690825