1 April 1992 Ultrafast Raman echo experiments in the liquid phase
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Abstract
The Raman echo experiment, which can distinguish homogeneous and inhomogeneous broadening of vibrational spectra, is reported for the first time in liquids. The symmetric methyl stretch of acetonitrile, which has been extensively studied with contradictory results, is shown to be homogeneously broadened. The vibration interacts only with rapid collisional motions of the solvent.
© (1992) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Mark A. Berg, Laura J. Muller, David A. Vanden Bout, "Ultrafast Raman echo experiments in the liquid phase", Proc. SPIE 1638, Optical Methods for Time- and State-Resolved Chemistry, (1 April 1992); doi: 10.1117/12.58168; https://doi.org/10.1117/12.58168
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