14 October 1997 Picosecond-milliangstrom resolution dynamics by ultrafast x-ray diffraction
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Abstract
Optical pump, x-ray diffraction probe measurements have been used to study the lattice dynamics of single crystals with picosecond-milliangstrom resolution by employing a table- top, laser-driven x-ray source. The x-ray source, consisting of an approximately 30 fs, 75 mJ/pulse, 20 Hz repetition rate, terawatt laser system and a moving Cu wire target assembly, generates approximately 5 X 1010 photons (4π steradians s)-1 of Cu Kα radiation. Lattice spacing changes of as small as 1 X 10-3 Å in a few picoseconds have been detected, utilizing Bragg diffraction from GaAs single crystals. Enhancement of the diffraction intensity associated with degradation of the crystals during and after the laser irradiation has been observed, likely due to a transition from dynamic to kinematic diffraction.
© (1997) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Ting Guo, Ting Guo, Christoph G. Rose-Petruck, Christoph G. Rose-Petruck, Ralph Jimenez, Ralph Jimenez, Ferenc Raksi, Ferenc Raksi, Jeffrey A. Squier, Jeffrey A. Squier, Barry Walker, Barry Walker, Kent R. Wilson, Kent R. Wilson, Christopher P. P. Barty, Christopher P. P. Barty, } "Picosecond-milliangstrom resolution dynamics by ultrafast x-ray diffraction", Proc. SPIE 3157, Applications of X Rays Generated from Lasers and Other Bright Sources, (14 October 1997); doi: 10.1117/12.283987; https://doi.org/10.1117/12.283987
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