Paper
11 June 2002 Exciton coherence in GaAs quantum wells probed by four wave mixing measurements at high excitation intensities
Bipul Pal, Arvind S. Vengurlekar
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Abstract
We perform two beam time integrated (TI) degenerate four wave mixing (DFWM) measurements on 8~nm GaAs quantum wells (QW). Pulses from a Ti-Sapphire laser resonantly excite only 1s heavy hole excitons. The power density of the leading pulse (I1) is increased, keeping that of the delayed pulse fixed and relatively small. We measure the TI-DFWM signal at different delays as well as the DFWM spectra at a fixed delay, as I1 is increased. We find that the dephasing rate, after an initial increase with I1, becomes independent of I1 for large I1. The spectrally integrated DFWM signal, which probes the coherent polarization of the resonantly excited QWs, initially increases with I1, reaches a peak and then decreases as 1/(root)I1 at large I1. The results are compared with theoretical models of exciton coherence.
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Bipul Pal and Arvind S. Vengurlekar "Exciton coherence in GaAs quantum wells probed by four wave mixing measurements at high excitation intensities", Proc. SPIE 4643, Ultrafast Phenomena in Semiconductors VI, (11 June 2002); https://doi.org/10.1117/12.470412
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KEYWORDS
Excitons

Quantum wells

Picosecond phenomena

Gallium arsenide

Polarization

Signal detection

Four wave mixing

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