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19 October 2004 An efficient nanolens: self-similar chain of metal nanospheres
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Abstract
As an efficient nanolens, we propose a self-similar linear chain of several metal nanospheres with progressively decreasing sizes and separations. To describe such systems, we develop the multipole spectral expansion method. Optically excited, such a nanolens develops the nanofocus (``hottest spot'') in the gap between the smallest nanospheres, where the local fields are enhanced by orders of magnitude due to multiplicative, cascade effect of its geometry and high $Q$-factor of surface plasmon resonance. The spectral maximum of the enhancement is in the near-ultraviolet, shifting toward the red as the separation between the spheres decreases. We also introduce surface plasmon amplification by stimulated emission of radiation (spaser) in nanolenses. Predominantly amplified are the dark, odd-parity eigenmodes, which do not suffer dipole-radiative losses and produce coherent, local optical fields comparable in strength to atomic fields, with minimal far-field radiation. The proposed systems can be used for nanooptical detection, Raman characterization, nonlinear spectroscopy, nano-manipulation of single molecules or nanoparticles, and other applications.
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Mark I. Stockman, Kuiru Li, Xiangting Li, and David J. Bergman "An efficient nanolens: self-similar chain of metal nanospheres", Proc. SPIE 5512, Plasmonics: Metallic Nanostructures and Their Optical Properties II, (19 October 2004); https://doi.org/10.1117/12.555743
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