Paper
25 November 1986 Effect On Beam Quality Of Lransient Refractive-Index Changes In Stimulated Raman Scattering
A. Flusberg, D. Korff
Author Affiliations +
Proceedings Volume 0642, Modeling and Simulation of Optoelectronic Systems; (1986) https://doi.org/10.1117/12.975491
Event: 1986 Technical Symposium Southeast, 1986, Orlando, United States
Abstract
Two sources of phase aberrations during amplification by stimulated Raman scattering have been studied. Both are caused by intensity nonuniformity in the incident pump laser beam. First, nonuniform population transfer of molecules undergoing the Raman transition results in a cumulative refractivity nonuniformity associated with the difference between the polarizabilities of the two molecular states. As shown experimentally by Butylkin et al. and Baklushina et al., the fractional polarizability difference for the Q(l) vibrational transition of H2 is ≈0.15-0.20. As a result, this effect becomes large at a fluence nonuniformity level >33/cm2. The dependence on fluence, rather than intensity, arises from the cumulative population transfer that takes place when the relaxation of the upper level during the laser pulse only weakly affects the population difference. Second, collisional relaxation of the excited population during the pulse causes heating and a nonuniform density distribution; this effect becomes more important as the pulselength is increased or the spatial scale size of the intensity gradients is decreased. The equations coupling the pump and Stokes fields to the refractivity and density changes are solved in the ray-optics limit of collimated beams and the effect on beam quality is determined. It is shown that in the limit of weak refractivity effects and negligible heating the beam-quality loss varies as the square of the rms fluence modulation.
© (1986) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
A. Flusberg and D. Korff "Effect On Beam Quality Of Lransient Refractive-Index Changes In Stimulated Raman Scattering", Proc. SPIE 0642, Modeling and Simulation of Optoelectronic Systems, (25 November 1986); https://doi.org/10.1117/12.975491
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KEYWORDS
Raman spectroscopy

Modulation

Collimation

Pulsed laser operation

Raman scattering

Optoelectronics

Phase shift keying

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