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Large crystals of Hg2Cl2 and Hg2Br2 (48 mm in diameter, up to 600g in weight) have been grown by self-seeded
contactless Physical Vapor Transport (PVT) technique in closed ampoules in vertical configuration. Seed selection
was accomplished in the small diameter tubing at the ampoule tip. Material purification was done by resublimation
processing. The crystals show high transparency, with good transmittance and good crystallographic quality. An
acousto-optic modulator built from the Hg2Cl2 crystal showed good performance consistent with predicted device
parameters.
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Joo-Soo Kim, Sudhir B. Trivedi, Jolanta Soos, Neelam Gupta, Witold Palosz, "Development of mercurous halide crystals for acousto-optic devices," Proc. SPIE 6661, Imaging Spectrometry XII, 66610B (12 September 2007); https://doi.org/10.1117/12.734102