18 May 2010 Towards a unifying theory for the first-, second-, and third-order molecular (non)linear optical response
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Abstract
We present a procedure for the modeling of the dispersion of the nonlinear optical response of complex molecular structures that is based strictly on the results from experimental characterization. We show how under some general conditions, the use of the Thomas-Kuhn sum-rules leads to a successful modeling of the nonlinear response of complex molecular structures.
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Javier Pérez-Moreno, Koen Clays, Mark G. Kuzyk, "Towards a unifying theory for the first-, second-, and third-order molecular (non)linear optical response", Proc. SPIE 7722, Organic Photonics IV, 772224 (18 May 2010); doi: 10.1117/12.854199; https://doi.org/10.1117/12.854199
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