8 August 2014 Soliton building from spontaneous emission by ring-cavity fiber laser using carbon nanotubes for passive mode locking
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We investigate the generation of a chirped pulse in a single-mode, ring-cavity, erbium-doped fiber laser employing carbon nanotubes (CNTs) as a saturable absorber (SA). The pulse propagation is simulated using analytical methods to understand and quantify the role of multiple SA properties, particularly in the propagation dynamics of the laser pulse. The soliton solution is obtained on the basis of nonlinear effects, such as gain dispersion, second anomalous group-velocity dispersion, self-phase modulation, and two-photon absorption for a generalized nonlinear Schrodinger equation. The influences of the SA parameter in the range from 0.1 to 0.4 on the chirp, power, and width of the soliton are calculated. A stable, passively mode-locked fiber laser using CNTs as an SA is modeled. In addition, the power, width, chirp, and phase of the soliton pulses can be tuned by choosing suitable SA parameters.



Single-wall carbon nanotubes (SWCNTs) have attracted much attention in the field of optical communications in recent years because of their ultrafast nonlinear optical properties in the near-infrared region arising from the saturation of excitonic transitions,12.3.4 their interesting electronic and optical properties, and several applications in photonics, which include nanometer-scale devices for light generation, photodetection, photovoltaic applications, and application as saturable absorbers (SAs).5,6 Recent developments in fiber lasers have led to a renewed interest in SAs. CNTs have emerged as a promising technology for the fabrication of SAs.7 Graphene89.10and nanoscale graphite11,12 materials based on CNTs have attracted much attention because of their high optical nonlinearity and fast recovery time when used as an SA in a mode-locked erbium-doped fiber laser (EDFL) for femtosecond/picosecond pulse generation.1314.

Because SWCNTs possess subpicosecond recovery times and broad absorption spectra, active fibers doped with Yb:KLuW operating at a wavelength of 1000 nm,19 a praseodymium-doped fiber operating at 1300 nm,20 a ytterbium-doped fiber operating at 1064 nm,21 and active fibers doped with Er+3 operating at 1500 nm have been mode-locked with SWCNT SAs.22

Most recent studies on fiber lasers have focused only on the use of CNTs with erbium (Er) fiber lasers for generating short optical pulses at a 22 MHz repetition rate with a 50 kW peak power and a 1.1 ps pulse width23,24 or a 39 MHz repetition rate with a 3.4 mW peak power and a 115 fs pulse width.25

In addition, new SA materials, such as TI:Bi2Se3 and TI:Bi2Te3, have attracted much attention for mode locking of an Er-doped fiber laser and have yielded stable soliton pulses of 1.57 ps at 1564.6 nm and 1.21 ps at 1558 nm, respectively.26,27 In 2014, Zhang developed an MoS2-based optical fiber SA device with an operation wavelength suitable for an ytterbium-doped fiber laser and experimentally generated nanosecond dissipative soliton pulses at 1054 nm.28

Most previous studies have been experimental, and few theoretical analyses in this field have been presented. Analytical methods may be useful for enabling the study of a wide range of SA parameters. An analytical study involves performing a spatial analysis to obtain new information; a spatial analysis would be difficult to perform experimentally. The theoretical description of pulse shaping and propagation in a fiber ring-cavity laser is based on the generalized nonlinear Schrodinger (NLS) equation. The Schrodinger equation can be solved either analytically or numerically. Analytical methods are more rigorous and provide exact solutions, but they are difficult to use for complex problems. Many articles have been published on the exact solutions to nonlinear wave equations. These include studies of the Backlund transform,29 the hyperbolic tangent expansion method,30 the trial function method,31 the nonlinear transform method,32 transformed rational function method,33 and exact 1-soliton solution of the complex modified Korteweg–de Vries equation method.34

Numerical methods, such as the split-step Fourier method, have become popular with the development of computing capabilities, although they only give approximate solutions of the NLS equation. 35 Previous studies of the exact solutions to nonlinear wave equations have not dealt with a range of SA parameters for CNTs.

In this paper, we describe and analyze a method for solving the NLS equation that involves the nonlinear effects of CNTs as an SA. The gain in the NLS equation is described by the saturation power of the gain medium, an average small-signal gain, and an average power over the cavity length. The rest of this paper is organized as follows. In Sec. 2, we derive the equations for representing the solitary wave. In Sec. 3.1, we discuss three cases for the chirp parameter and its effect on the generation of a soliton, and we investigate the effect of the SA parameter on the laser power, pulse phase, and pulse width. In Sec. 3.2, we focus on the chaotic behavior of the laser pulse. Section 3.3 considers the stability of the laser pulse; we focus on the phase of the pulse associated with the introduced transformations and present stationary solutions. In Sec. 3.4, we describe the effect of the SA parameter on the dynamic behavior of the chirped pulse.


Model Algebraic Equations

In this section, we describe the optical pulse propagation in a fiber laser using the NLS equation for the pulse envelope ψ(z,T) in the presence of mode locking with the use of an SA, including the gain dispersion, losses for the cavity and fiber, gain, group-velocity dispersion (GVD), self-phase modulation (SPM), and two-photon absorption (TPA). This equation can be written as5


where ψ(z,T) is the amplitude of the optical pulse, T is the time, z is the propagation distance, α is a coefficient that takes into account material losses in the cavity, δSA is the SA parameter, α2 is the TPA parameter, γ is the SPM parameter, β2 is the second-order dispersion coefficient, psatEr is the saturation power of the gain medium (Er+3), psatCNT is the saturation power of SA (CNTs), and gT22 is a frequency-dependent gain dispersion factor. We assume a chirped pulse given by






where ξ, σ, k, and c are four arbitrary parameters representing the amplitude, width, wave number, and chirp of the pulse, respectively.

When ψ/z is calculated using Eq. (2), it is found to satisfy



The first part of Eq. (5) is given by



The second part of Eq. (5) is given by



We can write an equation for the second derivative of Eq. (2) with respect to T after some algebra, as follows:



Let us assume the new parameters as





By calculating Γ/T and Ω/T, the result is given by





Substituting Eqs. (11) and (12) into Eq. (10), we obtain



We follow a similar procedure for finding the second derivative of Eq. (13):



Substituting Eqs. (2), (3), (4), (5), (6), (7), (13), and (14) into Eq. (1), after some algebra, we obtain the following equation:



Separating the real and imaginary parts of Eq. (15), we obtain the following two equations:





Equating the coefficient of sech2(σT) and other parameters in Eq. (16), we obtain the following equations:





Equation (17) can be separated into two equations in the form






Results and Discussion

The laser configuration consists of a ring cavity. Two types of fibers are used in the cavity: a 6-m piece of Er-doped fiber (EDF) and a standard single-mode fiber (SMF28) with a total net anomalous GVD β2 of 0.012ps2/m.

The gain in our fiber laser comes from the EDF, which, when pumped with 980-nm light, exhibits spontaneous emission at 1550 nm. Continuously pumping the gain fiber results in the formation of an initial pulse by amplified spontaneous emission, and the pulse makes several passes through the resonant cavity.36 It is important to fix the total length of the gain fiber so that the round trip time for a pulse through the resonant cavity basically equals the storage time of the gain fiber and the pulse will return on each successive pass to the gain fiber as the gain fiber has been pumped back up from a depleted state caused by the prior pass. A polarization-independent isolator was spliced into the cavity to force unidirectional operation of the ring. A CNT mode locker was placed between the EDF and the 10% fiber coupler, as shown in Fig. 1.

Fig. 1

Schematic of fiber laser components: Er-doped fiber (EDF), single-mode fiber, wavelength-division multiplexer, polarization controller, coupler, and optical isolator.



Chirp Dynamics

To understand the dynamic behavior of the chirp, Eqs. (19) and (21) can be used to find an equation for the chirp.



After some algebra, we obtain the following equation:



We can rewrite the above equation as


where the parameters m and n are given by



It is easy to show that the chirp parameter is





We can use Eq. (27) to investigate the chirp parameter; we discuss the three cases separately.

  • Case 1: The solution of Eq. (27) is called the symmetric state and exists only for m24n>0. The chirp parameter is real and indicates that the pulse-formed soliton will propagate without changes in its shape; the pulse is stable.

  • Case 2: When m24n=0, the chirp is given by c=m/2, indicating that the frequency is always shifted (chirping always occurs) unless the pulse forms a soliton.

  • Case 3: The solution of Eq. (27) represents an antisymmetric state and exists for all m24n<0. In this case, the chirp parameter is purely imaginary, and it is impossible to obtain the soliton from a pulse because the antisymmetric states are unstable.

From the condition that the chirp parameter is real, we obtain



For a fiber laser employing CNTs, gT22, β2, α2, g/psatEr, and γ play important roles in the evolution of passive mode-locked pulses and should be included.

According to Eq. (28), we obtain



When a complex number (β2+i(4/3)2gT22) is multiplied by its conjugate, the result is



The SA parameter δSA must be real; therefore, 4/32(β22g2T24)=0, and



This equation shows that the condition that the saturable absorption parameter δSA must yield a real chirp parameter c can be related to the stable soliton.

According to Eq. (21) and the condition |ξ|20, we obtain



This clearly illustrates that the nonlinear behavior is altered from saturable absorption to TPA as the intensity of the optical pulse increases. The transformation from saturable absorption to TPA suggests that another nonlinear process occurs and becomes dominant. This interesting effect can be used for optical pulse compression; the above behavior of the optical pulse depends on the values of the parameters gT22, β2, α2, δSA/psatCNT, g/psatEr, and γ.

We can use Eq. (27) to calculate the pulse chirp for δSA values between 0.1 and 0.4. Figure 2 shows the changes in the chirp as a function of δSA; the chirp increases linearly with δSA.

Fig. 2

Chirp versus saturable absorption parameter δSA.



Unstable Laser Pulse

Analytical simulations of pulses that grow through a 5-m fiber ring without a saturable absorption mode locker show that each input pulse develops an internal substructure consisting of many subpulses with widths on the order of femtoseconds. Figure 3 shows the evolution toward a parabolic shape when a “sech” pulse is amplified over the 5-m length of the fiber laser; the position and width of the subpulses change continuously in an apparently random manner. Changing the anomalous GVD values by varying the length of the SMF, therefore, will cause the total cavity dispersion to vary as well.37 Figure 3 shows that each pulse still develops an internal substructure that depends on the frequencies of the photon laser through the ring resonator, and the pulse power also varies from pulse to pulse and exhibits chaotic behavior as the phase is varied in the cavity resonance.

Fig. 3

Evolution of substructure in a 5 m ring resonator when pulses grow from spontaneous emission with group-velocity dispersion: (a) β2=0.014ps2/m, (b) β2=0.012ps2/m. Other parameters are γ=0.012(Wm)1, α2=0.3, T2=0.047ps, α=0.17823m1, and g=0.78275m1.



Stable Pulse (Soliton)

The solution of Eq. (2) provides a shortcut to understanding the behavior of pulse laser propagation through an Er+3 ring cavity 6 m in length with a saturable absorption mode locker. In this section, we concentrate on the effects of the absorption parameter on the characteristics of the laser pulse; the absorption parameter is tuned in a wide range from 0.1 to 0.4 (Ref. 38) by varying the thickness of the CNTs. First, by joining Eqs. (20) and (27), we find the soliton width σ. Second, from Eq. (18), we obtain the wave number of the soliton, k. Third, from Eq. (21), we can obtain the soliton power. Fourth, we substitute the soliton width, soliton power, and wave number into Eqs. (3) and (4) and algebraically combine the resulting equations with Eq. (2) to obtain a solitary wave equation describing the dynamics and propagation of optical pulses in a 6-m-long EDFL.

Figure 4 shows the three-dimensional soliton pulse propagation in an EDFL, and Fig. 5 shows the sech pulse profile when the system parameters are γ=0.012(Wm)1, β2=0.012  ps2/m, α2=0.3, T2=0.047ps, δSA=0.1, α=0.178m1, psat=210W, and g=0.782m1.38 The power of the soliton grows exponentially once the power of the pulse exceeds a threshold value, where, at z=10cm, the power of the soliton is 0.007 W, and a picosecond optical pulse is amplified in the EDFL until the gain saturates at z=4m with a power of 1.2 W.

Fig. 4

Soliton growth from spontaneous emission with erbium-doped fiber laser parameters of γ=0.012(Wm)1, β2=0.012ps2/m, α2=0.3, T2=0.047ps, α=0.17823m1, g=0.78275m1, δSA=0.1 and psat=210W.


Fig. 5

Profiles of parabolic pulse at (a) z=0.1m and (b) z=6m.


Figures 6(a) and 6(b) show the variation in the soliton phase with time and with the length of the fiber laser, respectively, according to the phase equation φ=kzclog[cosh(σT)], for a fixed length of z=4m. The phase changes with time as a cosine wave with a range of 1 to 1, as shown in Fig. 6(a). The wave number k; in the phase equation depends on β2, gT22, c, and TFWHM, as shown in the following equation:





Fig. 6

Soliton phase plotted as a function of (a) time and (b) fiber length.


Let us consider the case in which the soliton phase varies linearly along the fiber length, as shown in Fig. 6(b). At z=0m, the soliton phase is φ=0.7, and the phase reaches a maximum value of φ=0.57 when z=6m. Clearly, the values of the phase play an important role in building the soliton from spontaneous emission of the Er+3 fiber laser.


Effect of SA on Soliton Behavior

First, we explain the control of the pulse width in a mode-locked fiber laser in which CNTs act as an SA by adjusting the laser’s intracavity SA parameter. Equation (35) shows that the SA parameter can vary with TFWHM.



Figure 7(a) shows the soliton width (FWHM) as a function of δSA. The soliton width increases with δSA.

Fig. 7

(a) width of soliton and (b) output power versus δSA.


Second, we focus on the soliton power and SA parameter. Increasing δSA reduces the soliton power, as can be inferred from Eq. (36). Furthermore, it is easy to show that δSA depends on psat and p and refers to the evolution of the building pulse toward a soliton as its width decreases and peak power increases, as shown in Fig. 7(b).



Figures 8(a) and 8(b) show the effect of changing the δSA on the shape of the soliton; the soliton is repeatedly propagated around the laser cavity until a steady state is reached. The soliton power grows exponentially along the fiber length. SAs can also be used to filter sidebands associated with solitons because sidebands can be selectively transferred to the lossy core because of their low power level.

Fig. 8

Soliton growth from spontaneous emission: (a) δSA=0.2, (b) δSA=0.3.


The soliton power in the fiber resonators is evident from Eq. (37). Note that the power depends on the GVD β2, gain dispersion gT22, chirp c, SPM parameter γ, and soliton width TFWHM.





It is evident from Eqs. (37) and (38) that the parameters ξ and TFWHM can have real, positive values or imaginary values, depending on the value under the radical of Eq. (38). ξ and TFWHM play an important role in stable optical pulses; if ξ and TFWHM are real, the optical pulse forms a soliton. Figures 9(a) and 9(b) show that the output pulse forms a soliton and becomes broader with increasing δSA and decreasing power.

Fig. 9

Profile of optical pulse that forms a soliton for (a) δSA=0.2 and (b) δSA=0.3.




We highlighted four important properties: the power, width, chirp, and phase of the pulse laser on the basis of a mathematical model for fiber lasers with ring cavities and CNTs as an SA mode locker. For values of γ=0.012(Wm)1, β2=0.012ps2/m, α2=0.3, T2=0.047ps, α=0.17823m1, g=0.78275m1, and psat=210W, ξ and TFWHM must be positive and real to guarantee stable pulse propagation (a soliton). In this paper, we argued that δSA=0.1 is the best value for generating solitons at a power of 1.2W and width of 0.5ps. The second major finding was that the soliton power decreases as the SA parameter δSA increases, but that the soliton width increases with increasing δSA. Furthermore, different δSA values yield different soliton characteristics; this provides a convenient method for tuning the properties of the generated soliton in ring-cavity fiber lasers, where the properties of the SA parameter depend on the size of the CNTs; therefore, the TPA from a thinner diameter of the CNTs could destroy the stability of mode-locked pulse formation. Consequently, a thicker diameter of the CNTs with less nonlinearity was identified as the mode locker to reduce the TPA, where both gain dispersion and two-photon absorption provide such a loss mechanism, and hence, the TPA plays an important role in establishing the soliton. These observations are in agreement with numerical simulations.38 Moreover, our results for the parabolic shape of the pulse and the behavior of the laser pulse propagation through the fiber laser exhibit good agreement with previous studies.3940.41.42.43


The author is grateful for the assistance of Professor Dr. Kavintheran Thambiratnam and Professor Dr. Zoltan Varallyay.


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Younis Mohamed Atiah Al-zahy has been an associate professor of physics in the Department of Science at Misan University since 2006. He received a PhD and MSc degrees in the College of Physical Science from Al-Mustansiriya University, Iraq, in 2006 and 1998, respectively. Currently, he works at the Laboratory of Laser Technology, and the College of Science as a lecturer in physics. He has published many papers in the field of fiber lasers.

© The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License. Distribution or reproduction of this work in whole or in part requires full attribution of the original publication, including its DOI.
Younis Mohamed Atiah Al-zahy, Younis Mohamed Atiah Al-zahy, } "Soliton building from spontaneous emission by ring-cavity fiber laser using carbon nanotubes for passive mode locking," Optical Engineering 54(1), 011005 (8 August 2014). https://doi.org/10.1117/1.OE.54.1.011005 . Submission:


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