Spectroscopic holography refers to techniques in which the detected hologram contains information about specific species in the medium under study. In general, at least two lasers are required with wavelengths chosen carefully to fit the interaction process utilized. In this process, energy from the shorter wavelength laser beam is transferred to the longer wavelength coherently through the process of stimulated emission. Two interaction mechanisms are considered; Stimulated Laser Induced Fluorescence (LIF) and Stimulated Raman Scattering (SRS), which both are species specific with the ability of coherent interaction. In this paper, the fundamental properties of spectroscopic holography is presented and demonstrated with a few idealized experiments. These validation experiments are performed in a gas chamber in which different gases may be blended and the gas pressure changed between 1-12 bars. In addition, two examples of applications are presented. In the first set of experiments, LIF holography is used to image light absorption and laser heating in a dye simultaneously. The second set of experiments is performed in a ow of methane gas. It is demonstrated that the combination of holographic phase measurements and SRS gain images may be used for calibration. This calibration may further be used to measure absolute concentration in a burning flame.
In this paper a single-shot digital holographic set-up with two orthogonally polarized reference beams is proposed to achieve rapid acquisition of Magneto-Optical Kerr Effect images. Principles of the method and the background theory for dynamic state of polarization measurement by use of digital holography are presented. This system has no mechanically moving elements or active elements for polarization control and modulation. An object beam is combined with two reference beams at different off-axis angles and is guided to a detector. Then two complex fields (interference terms) representing two orthogonal polarizations are recorded in a single frame simultaneously. Thereafter the complex fields are numerically reconstructed and carrier frequency calibration is done to remove aberrations introduced in multiplexed digital holographic recordings. From the numerical values of amplitude and phase, a real time quantitative analysis of the polarization state is possible by use of Jones vectors. The technique is demonstrated on a magnetic sample that is a lithographically patterned magnetic microstructure consisting of thin permalloy parallel stripes.
The stimulated Raman scattering (SRS) signal in diffuse light has been recorded using an optical imaging technique based on spatial modulation. A frequency doubled Q-switched Nd-YAG laser (wavelength 532 nm) has been used to pump a polymethyl methacrylate (PMMA) cylinder. The frequency tripled (355 nm) beam from the same laser is used to pump an optical parametric oscillator (OPO). The Stokes beam (from the OPO) has been tuned to 631.27 nm so that the frequency difference between the pump and the Stokes beams fits a Raman active vibrational mode of the PMMA molecule (2956 cm<sup>-1</sup>). The two laser beams were overlapped in time and space on a PMMA cylinder resulting in a gain of the Stokes beam through the SRS process of about 4.0 %. For separating the SRS signal, the pump beam was spatially modulated with fringes produced in a Michelson interferometer. The gain of the Stokes beam due to SRS was separated from the Stokes beam background in the Fourier domain. The intensity image has been calculated from an inverse Fourier transform of the separated gain signal. The intensity image shows a gain of the Stokes beam at the area of overlap between the pump beam fringes and the Stokes beam compared to the undisturbed surrounding. The results show that spatial modulation of the pump beam is a promising method to separate the weak SRS signal from the Stokes beam background. This technique can be applied to pin-point specific species and record its spatial and temporal distribution.
A frequency tripled Q-switched Nd-YAG laser (wavelength 355 nm, pulse duration 12 ns) has been used to pump
Coumarin 153 dye solved in ethanol. The laser induced fluorescence (LIF) spectrum has been recorded using a
spectrometer at different dye concentrations. The frequency doubled 532 nm beam from the same laser is used as a probe
beam to pass through the excited volume of the dye. Because of stimulated emission an increase of the probe (532 nm)
beam energy is recorded and a reduction of the spontaneous fluorescence spectrum intensity is observed. A model was
developed that approaches the trend of the gain as a function of the probe beam energy at low dye concentrations (less
than 0.08 g/L). The stimulated LIF is further recorded using digital holography. Digital holograms were recorded for
different dye concentrations using collimated laser light (532 nm) passed through the dye volume. Two holograms
without and with the UV laser beam were recorded. Intensity maps were calculated from the recorded digital holograms and are used to calculate the gain of the green laser beam due to the stimulated fluorescence emission which is coupled to the dye concentration. The gain of the coherent 532 nm beam is seen in the intensity maps and its value is about 40% for a dye concentration of 0.32 g/L and decreases with the decrease of the dye concentration. The results show that pulsed digital holography can be coupled to the stimulated LIF effect for imaging fluorescent species.