Fabrication of all-solid-state Li battery has been strongly required to overcome safety issue of present Li battery. One of
promising structures for ceramics electrolyte in all-solid-state battery is 2-layered structure composed of 3 dimensionally
ordered macroporous layer (3DOM) and dense layer. In this study, we prepared Li0.35La0.55TiO3 (LLT) ceramics
electrolyte with the 2-layered structure by suspension filtration method. Thicknesses of the dense and the porous layers
were about 23 and 105 μm, respectively. The porous layer involved uniform pores of 1.8 μm in diameter. An
electrochemical property of LiMn2O4 / 2-layered LLT composite, prepared by impregnation of precursor sol for
LiMn2O4 into the pores followed by calcination, was tested. A rechargeable behavior of the composite electrode was
clearly observed. From this result, it can be said that the composite can work as rechargeable battery. The discharge
capacity of the composite was 27 mA h g-1.
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