The instrument set-up designed by the PreViBOSS project for the ParisFog field campaign is suitable to sound microphysical properties of droplets and interstitial aerosols during developed fog in a semi-urban environment. Developed fog is defined as LWC < 7 mg m-3 and the temperature vertical gradient over 30 m, ΔT, smaller than 0.04 K/m. Visibility averaged over November 2011 is 385±340 m (with rare values larger than 1000 m), and month average of LWC is 60±60 mg m-3. The droplet effective radius decreases from 14 to 4 μm when the number concentration increases from less than 10 to 220 cm-3. Particle extinction coefficient is computed by Mie theory applied on size distribution observed during developed fog in ambient conditions by both PALAS WELAS and DMT FM100. Comparison with particle extinction coefficient directly measured by the Degreanne DF20 visibilimeter demonstrates satisfying agreement, within combined uncertainties. Ratio of computed over measured particle extinction coefficient is 1.15±0.35. Visibility smaller than 1000 m at 3 m above ground level is observed not only during developed fog but also during shallow fog, which presents a significant vertical gradient, as ΔT > 0.4 K/m. In this case, LWC is highly variable and may be observed below 7 mg m-3. The consequent month average of LWC is 30±80 mg m-3. The optical counters miss large droplets significantly contributing to extinction in shallow fogs. Consequently, it is not possible to reproduce with satisfaction the particle extinction coefficient in shallow fog. Fog type may be distinguished by association of groundbased visibilimeter and MSG/SEVIRI. When clear-sky is given by EUMETSAT/NWCSAF cloud type product while visibility is observed smaller than 1000 m at SIRTA, in 75% cases a shallow fog occurs, and in other cases, horizontal heterogeneity characterises the developed fog within the SIRTA pixel, as during the dissipation phase. Moreover, consistently, low and very low clouds are mostly detected by the satellite product when developed fog is observed by ground-based instrumentation.
Aerosol optical properties are retrieved from measurements acquired during the 2003 summer at the new AERONET station of Evora, Portugal, with a sun/sky photometer, a fluxmeter and a nephelometer. Aerosol optical thickness (aot) derived at several wavelengths shows that an exceptionally long turbid event occurred in July-August. Desert dust particles transported from North Africa increased aot at 873 nm (aot873) to the value of 0.27 with an Ångstrom exponent αC=0.5. Emissions from forest fires in The Iberic peninsula affected Evora since the end of the dust episode, with aot441 reaching 0.81 and aC=1.8. The aerosol scattering coefficient measured at surface level shows that desert dust does not reach the surface level at Evora while the forest fire emissions were uniformly distributed over the atmospheric column. Sky-radiance and flux measurements agree in retrieval of the aerosol single scattering albedo (assa) at several wavelengths. A large absorption rate is found with a high spectral dependence for desert dust particles (assa441=0.86 and ass873=0.93) and with a flat spectral dependence during the forest fires emission episode (assa441=0.88 and assa873=0.87). All measurements as well as back-trajectory calculations indicate mixture of particles during the desert dust.
A 'measure’ of the surface effect on downwelling radiance in the solar principal plane (SPP), K, is built by analysing simulations by a radiative transfer code. K describes the solar angle dependence of the radiance measured at a viewing angle θv=40° over radiance measured at θv=70°, both in SPP. The surface effect is described by a surface albedo value, used as an input parameter of the Successive Orders of Scattering code [Deuze et al., 1989]. K is mainly sensitive to the surface albedo but also to the Ångström exponent α and to the real part of the refractive index mR. α is derived from independent measurements of spectral aerosol optical thickness and mR is estimated in a first step of the method from radiance measurements made at θSun=70°. The method is applied on data acquired at the AERONET site of Sede Boker, Israel, in 2000. Results give a high reflective surface with small spectral dependence. An event of increase of vegetation cover (which we suppose is caused by rain falls) is observed as the surface albedo at 675 nm decreases while it remains constant at 870 nm. Aerosol single scattering albedo derived at 675 nm from radiance measurements varies little around 0.90 only if surface albedo change is considered.
Multi-angle multi-spectral scans of upward total and polarized radiance were measured by the Research Scanning Polarimeter onboard a Cessna 210 aircraft during the Chesapeake Lighthouse and Aircraft Measurements for Satellites experiment. The surface contribution to the polarized radiance (PR) was evaluated for its effect on the retrieval of aerosol properties from PR over land surfaces. The atmospheric contribution to PR was negligible at 2250 nm for an aerosol having an aerosol optical thickness (AOT) at 440 nm of 0.72 and AOT at 865 nm of 0.17. The atmospheric and surface contribution to PR at 865 nm were found to be similar for this aerosol load. Thus, although the 2250 nm measurements can be used to characterize the surface on this very turbid day, this is not the case for the 865 nm measurements. The polarized and total radiances at 1590 and 2250 nm were found to be strongly correlated, suggesting that a common physical process affects reflection and polarization since this correlation was present even within a given surface type. Near the backscattering direction a simple front facet Fresnel reflection model of surface polarization breaks down and the surface polarized reflectance shows considerable spectral variability and angular structure that may be of use in evaluating the structural parameters of vegetated and soil surfaces.
An important source of uncertainty in radiative forcing of climate models is their treatment of tropospheric aerosols. Satellite radiometry offers the only means of providing aerosol characterization on a global scale. POLDER (POLarization and Directionality of the Earth's Reflectances) instrument was launched in August 1996 on the ADEOS platform. Aerosol products are derived from combination of multiangular, multispectral and polarized observations in visible and near infrared bands. Validation effort has been planned to test POLDER aerosol products by comparison to independant measurements. The validation is achieved using ground based sunphotometers from a worldwide station network and by performing or participating to specific campaign such as ACE-2 (Aerosol Characterization Experiment) for marine and desert dust aerosol, AMT-4 (Atlantic Meridian Transect) with a ship crossing from Falklands to England (marine aerosol) and to continental campaigns in France (urban and continental aerosol). In the paper, two aspects of the validation will be presented. The first point concerns the analysis of data acquired during the specific campaigns. In that case, sunphotometer and polarimeter measurements will be qualitatively analysed but also used into comparison with POWER model database. In a second step, we shall report systematic studies of the worldwide sunphotometer network measurements (statistic on aerosol loading, Angstrom coefficient related to particle size). First results of these statisical studies will be presented and will be taken into account in the aerosols model database used into the POLDER aerosol algorithm. Keywords: POLDER, aerosols, polarization, validation.
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