In this paper we report on fabrication of a nanocomposite based on CdSe quantum dots mixed with commercial photoresist ORMOCOMP and proved its high structurability by direct laser writing. The distribution of quantum dots was visualised by transmission electron microscopy and the quality and geometrical parameters of the structures were studied by optical and atomic force microscopy. We manufactured a novel photonic device for Bloch surface electromagnetic waves in photonic crystals and thoroughly studied their propagation by both leakage microscopy and back focal plane imaging methods. By z-scan method we measured the nonlinear Kerr coefficient of quantum dots. Its high value makes the manufactured photonic device promising for all-optical switching applications.
We have studied an influence of Tamm plasmon-polaritons (TPPs) excitation on the nonlinear-optical response of one-dimensional photonic crystal/metal structures. It was shown that in case when the fundamental radiation is in resonance with the TPP, second-harmonic generation in the sample is enhanced over two times of magnitude in comparison with a bare metal film. Using methods of nonlinear transfer matrices it was demonstrated that the third-order nonlinear response of a metal/dielectric heterostructure, when both fundamental and third-harmonic radiation are in resonance with the first- and third-order TPPs respectively, can be enhanced via two mechanisms: fundamental field localization and optical harmonic resonant tunneling. The overall enhancement of the third harmonic generation in that case can exceed three orders of magnitude in comparison with the non-resonant case.
Temporal profile distortion of a femtosecond pulse reflected from one-dimensional plasmonic crystal have been
studied using time-resolved cross-correlation technique. Spectral dependences of cross-correlation functions show
that SPP resonance with Fano-type lineshape strongly disturbs reflected pulse on picosecond timescale.