Dispersive Fourier method gives access to spectral information by mapping them in the time domain. This facilitates shot-to-shot spectroscopy of rapidly changing systems. We adapted this technique to demonstrate time-resolved THz spectroscopy at 50 kHz repetition rate by encoding the THz waveform onto the spectral components of spectrally broadened (NIR) ultrafast laser pulses.
The rapid acquisition of terahertz (THz) time-domain waveforms is a significant challenge in the study of fast and non-reproducible phenomena. To increase data acquisition rates, the THz waveform can be encoded on spectral components of individual near-infrared (NIR) ultrafast laser pulses. By using dispersive Fourier transform method, where spectral information are mapped in the time domain, we demonstrate time-resolved THz-spectroscopy at an unprecedented rate of 50 kHz. With this technique, we resolve sub-millisecond dynamics of carriers in silicon injected by successive resonant pulses as a saturation density is established.
Terahertz time-domain spectroscopy (THz-TDS) is a method used in research and industry for non-invasive characterization of products and materials. Many THz-TDS systems rely on parametric conversion in semiconductor crystals to generate and detect phase-locked THz pulses, providing reliable access to frequencies below 3 THz. Accessing higher frequencies, however, often requires a sophisticated near-infrared (NIR) source delivering sub- 100 fs pulses to access the required spectral bandwidth and thin nonlinear crystals (few hundred micrometers thick) to minimize phase mismatch during both the THz generation and detection processes. As a result, broadband THz- TDS configurations rely on laser systems which are often bulky and costly, resulting in inefficient THz generation and detection processes due to a limited nonlinear interaction length in the crystals. To overcome these limitations, we introduce three modules to a THz-TDS system employing a compact and cost-effective pulsed laser. First, a fiberbased component is used to broaden the output laser spectrum and compress the pulse duration. This module provides the NIR frequency content needed for broadband THz generation through optical rectification and a pulse duration short enough to efficiently resolve high THz frequencies during electro-optic sampling. The other two modules utilize a thick nonlinear crystal with a periodically patterned surface to optimize the efficiencies of the broadband THz generation and detection processes. In this configuration, a long nonlinear interaction length is guaranteed while noncollinear phase matching provides access to a broad spectral range. The combination of these modules extends the THz spectrum from 3 THz to beyond 6 THz with a peak dynamic range >50 dB at 3.5 THz.
We report on the experimental demonstration of nonlinear spectroscopy of crystalline quartz in the terahertz regime. Using accumulated time shift method in the time domain, we observe that with increasing the THz pulse intensity, the experienced delay increases. At higher field intensities, the delay increases with a smaller rate, demonstrating a phase saturation. Analysing the frequency response, we estimate a nonlinear refractive index of the order of 10−13 m2/W which exceeds its value in the visible range by seven orders of magnitude. Furthermore, a negative fifth-order susceptibility of the order of 10−30 m4/V4 is obtained.
Many-body correlation effects in complex quantum systems often lead to phase transitions that bear great technological potential. However, the underlying microscopic driving mechanisms or even the quantum-mechanical properties of the novel ground state often remain elusive. Here we employ phase-locked ultrabroadband terahertz (THz) pulses to disentangle two coexisting orders in the charge density wave phase 1T-TiSe2 via their individual non-equilibrium multi- THz dynamics. Furthermore, we demonstrate that few-cycle THz pulses can project out the matter part of a transient cold exciton-polariton condensate, providing novel insights into the very nature of this macroscopic quantum state.
We report results from a systematic study of the linear refractive
index of thin films made of As-S-Se glasses which are part of
the chalcogenide family. We have studied eight different
compositions. The refractive index are measured by the mean of a
grating coupling experiment. The measurements are performed around
1.5μm for both annealed and non-annealed glasses. We observe
that annealing the samples increases their refractive index. We
also note that the increase of Selenium concentration increases
the refractive index and the decrease of Arsenic concentration
decreases the refractive index.
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