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5 March 2022 Progress in the optical response of crystalline atomically thin films
Álvaro Rodríguez Echarri, Joel D. Cox, Fadil Iyikanat, F. Javier García de Abajo
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Proceedings Volume PC12003, 2D Photonic Materials and Devices V; PC120030K (2022) https://doi.org/10.1117/12.2609481
Event: SPIE OPTO, 2022, San Francisco, California, United States
Abstract
Recent progress in the fabrication of metallic thin films allows for a precise control of the surface crystallographic orientation and thickness, turning them to be a great appeal in plasmonic devices. Considering such a crystalline quality and going towards smaller optical designs; surface, nonlocal, and quantum finite-size effects play a major role in metallic thin films when interacting with light. Here we explore various strategies to seek for the linear and nonlinear optical response manifested in a variety of scenarios and configurations which are based on precise quantum-mechanical formalisms that describe the dynamics of electrons in such films, e.g. EELS, Feibelman d-parameters, periodic- and finite-systems, etc. We believe that our results can inspire future devices based on crystalline metal films as well as motivate further numerical implementation strategies.
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Álvaro Rodríguez Echarri, Joel D. Cox, Fadil Iyikanat, and F. Javier García de Abajo "Progress in the optical response of crystalline atomically thin films", Proc. SPIE PC12003, 2D Photonic Materials and Devices V, PC120030K (5 March 2022); https://doi.org/10.1117/12.2609481
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KEYWORDS
Crystals
Crystal optics
Nonlinear crystals
Plasmons
Electrons
Near field optics
Photonic crystals
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