The vapor or gas-phase synthesis methods (e.g., CVD) are widely adopted to grow mono and few-layer two-dimensional (2D) materials. However, uncontrolled gas-phase reactions, complex flow dynamics, and limited reproducibility have made the gas phase growth of monolayer TMDCs crystals extremely challenging. Here we introduce a novel laser-assisted synthesis method for the rapid growth of various 2D materials. To produce the atomically-thin crystals, instead of using conventional multi-component precursors, this synthesis method utilizes stoichiometric powders as precursors that are laser vaporized to create the right vapor flux for the controlled growth of mono and few-layer crystals. We demonstrate a successful synthesis of four semiconducting TMDC monolayers such as MoS2, MoSe2, WSe2, and WS2 crystals. This laser vaporization process promises an efficient general synthesis solution for the accelerated growth of a variety of high-quality 2D quantum materials.
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