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In this talk we show how time-resolved Raman spectroscopy can be combined with Time Correlated Single Photon Counting (TCSPC) to create and evidence entanglement between light and a collective molecular vibration (i.e. an optical phonon) [3]. We further show that the correlations are strong enough to violate the Bell Inequality, which provides the most stringent test for entanglement. We measure the decay of these hybrid photon-phonon Bell correlations with sub-picosecond time-resolution and find that they survive over several hundred oscillations at ambient conditions.
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Christophe Galland, Santiago Tarrago Velez, Vivishek Sudhir, Anna Pogrebna, Nicolas Sangouard, "Bell correlations between light and vibrations in diamond at ambient conditions," Proc. SPIE 11806, Quantum Nanophotonic Materials, Devices, and Systems 2021, 118060E (1 August 2021); https://doi.org/10.1117/12.2594132