Open Access
11 April 2020 Spatiotemporal rotational dynamics of laser-driven molecules
Kang Lin, Ilia Tutunnikov, Junyang Ma, Junjie Qiang, Lianrong Zhou, Olivier Faucher, Yehiam Prior, Ilya Sh. Averbukh, Jian Wu
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Abstract

Molecular alignment and orientation by laser fields has attracted significant attention in recent years, mostly due to new capabilities to manipulate the molecular spatial arrangement. Molecules can now be efficiently prepared for ionization, structural imaging, orbital tomography, and more, enabling, for example, shooting of dynamic molecular movies. Furthermore, molecular alignment and orientation processes give rise to fundamental quantum and classical phenomena like quantum revivals, Anderson localization, and rotational echoes, just to mention a few. We review recent progress on the visualization, coherent control, and applications of the rich dynamics of molecular rotational wave packets driven by laser pulses of various intensities, durations, and polarizations. In particular, we focus on the molecular unidirectional rotation and its visualization, the orientation of chiral molecules, and the three-dimensional orientation of asymmetric-top molecules. Rotational echoes are discussed as an example of nontrivial dynamics and detection of prepared molecular states.

CC BY: © The Authors. Published by SPIE under a Creative Commons Attribution 4.0 Unported License. Distribution or reproduction of this work in whole or in part requires full attribution of the original publication, including its DOI.
Kang Lin, Ilia Tutunnikov, Junyang Ma, Junjie Qiang, Lianrong Zhou, Olivier Faucher, Yehiam Prior, Ilya Sh. Averbukh, and Jian Wu "Spatiotemporal rotational dynamics of laser-driven molecules," Advanced Photonics 2(2), 024002 (11 April 2020). https://doi.org/10.1117/1.AP.2.2.024002
Received: 21 January 2020; Accepted: 11 March 2020; Published: 11 April 2020
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CITATIONS
Cited by 33 scholarly publications.
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KEYWORDS
Molecules

Molecular lasers

Polarization

Picosecond phenomena

Polarizability

Pulsed laser operation

Photonics

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