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We present pump-probe and Raman measurements on individual plasmonic nano-junctions. The time-resolved measurements reveal differences between capacitive and conductive junctions, and paint a detailed picture of the ultrafast electrodynamics of the nano-junction. The insights gleaned from these measurements help interpret the ultrafast response of single molecules placed in the junction.
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Eric O. Potma, Alexander Fast, Kevin T. Crampton, Vartkess A. Apkarian, "Ultrafast pump-probe and Raman experiments of individual plasmonic junctions (Conference Presentation)," Proc. SPIE 10380, Ultrafast Nonlinear Imaging and Spectroscopy V, 103800O (19 September 2017); https://doi.org/10.1117/12.2274509